功能高分子材料教育部重点实验室

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刘遵峰课题组 | ACS APPLIED MATERIALS & INTERFACES

发布人:功能高分子材料教育部重点实验室    发布时间:2019/04/11   浏览次数: 次

Controllable Preparation of Ordered and Hierarchically Buckled Structures for Inflatable Tumor Ablation, Volumetric Strain Sensor, and Communication via Inflatable Antenna

Wang, R (Wang, Run)[ 1,2 ] ; Liu, ZS (Liu, Zhongsheng)[ 1,2,3 ] ; Wan, GY (Wan, Guoyun)[ 4 ] ; Jia, TJ (Jia, Tianjiao)[ 1,2 ] ; Zhang, C (Zhang, Chao)[ 5,6 ] ; Wang, XM (Wang, Xuemin)[ 7,8 ] ; Zhang, M (Zhang, Mei)[ 9 ] ; Qian, D (Qian, Dong)[ 7,8 ] ; de Andrade, MJ (de Andrade, Monica Jung)[ 8 ] ; Jiang, N (Jiang, Nan)[ 1,2 ] ; Yin, SG (Yin, Shougen)[ 10 ] ; Zhang, R (Zhang, Rui)[ 7,8 ] ; Feng, DQ (Feng, Deqiang)[ 1,2 ] ; Wang, WC (Wang, Weichao)[ 1,2 ] ; Zhang, H (Zhang, Hui)[ 8] ; Chen, H (Chen, Hong)[ 3 ] ; Wang, YS (Wang, Yinsong)[ 4 ] ; Ovalle-Robles, R (Ovalle-Robles, Raquel)[ 11 ] ; Inoue, K (Inoue, Kanzan)[ 11 ] ; Lu, HB (Lu, Hongbing)[ 7,8 ] ; Fang, SL (Fang, Shaoli)[ 8 ] ; Baughman, RH (Baughman, Ray H.)[ 8 ] ; Liu, ZF (Liu, Zunfeng)[ 1,2 ] 

ACS APPLIED MATERIALS & INTERFACES, 2019, 11(11): 10862-10873

DOI: 10.1021/acsami.8b19241

Abstract

Inflatable conducting devices providing improved properties and functionalities are needed for diverse applications. However, the difficult part in making high-performance inflatable devices is the enabling of two-dimensional (2D) buckles with controlled structures on inflatable catheters. Here, we report the fabrication of highly inflatable devices with controllable structures by wrapping the super-aligned carbon nanotube sheet (SACNS) on the pre-inflated catheter. The resulting structure exhibits unique 2D buckled structures including quasi-parallel buckles, crisscrossed buckles, and hierarchically buckled structures, which enables reversible structural changes of 7470% volumetric strain. The 2D SACNS buckled structures show stable electrical conductance and surface wettability during large strain inflation/deflation cycles. Inflatable devices including inflatable tumor ablation, capacitive volumetric strain sensor, and communication via inflatable radio frequency antenna based on these structures are demonstrated.